Dust aerosols play a critical role in atmospheric processes, influencing air quality, climate, and weather patterns through their interactions with radiation and cloud formation. This study aimed at characterizing the spatiotemporal distribution of dust and quantifying its radiative forcing over Kenya using a combination of satellite observations and model-based measurements. Multi-year datasets from MERRA-2 and MODIS were utilized to analyze dust loading and spatial variability. Additionally, radiative forcing (RF) derived from MERRA-2 and satellite observations was estimated to assess dust-induced changes in surface of-atmosphere (BOA), top-of-atmosphere (TOA) and within atmosphere (ATM). The findings on spatiotemporal variability of dust over Kenya, highlight high concentrations in northern regions during dry months and reductions during wet seasons (MAM and OND). While on particle size distribution, the analysis shows coarse-mode dominance in dry periods, depicting dominance of dust. On the other hand, dust mass concentrations peak in the northwest part of the study domain. Further, RF analysis indicates dust induces BOA and TOA cooling but atmospheric heating, with peak heating in June to July, local dry months. This study therefore recommends an enhanced integrated dust monitoring and modeling system, especially during dry seasons, to capture Dust AOD, size, and mass concentration. Further, targeted mitigation measures like afforestation, land-use planning and early warning systems should be prioritized to reduce dust emissions, improve climate model accuracy, and protect public health in vulnerable regions.
KeywordsCharacterizationDustAODRadiative ForcingSize Distribution
IPCC (2013) Climate Change 2013: The Physical Science Basis. Contribution of Working Group-I to the Fifth 4 Assessment Report of the Intergovernmental Panel on Climate Change. Cambridge University Press, 1535. https://doi.org/10.1017/CBO9781107415324
Intergovernmental Panel on Climate Change (IPCC) (2023) Climate Change 2021—The Physical Science Basis. Cambridge University Press. https://doi.org/10.1017/9781009157896
Seinfeld, J.H., Pandis, S.N. and Noone, K. (1998) atmospheric Chemistry and Physics : From Air Pollution to Climate Change . Physics Today , 51, 88-90. https://doi.org/10.1063/1.882420
Tang, R., Lu, Q., Guo, S., Wang, H., Song, K., Yu, Y., et al. (2021) Measurement Report: Distinct Emissions and Volatility Distribution of Intermediate-Volatility Organic Compounds from On-Road Chinese Gasoline Vehicles: Implication of High Secondary Organic Aerosol Formation Potential. Atmospheric Chemistry and Physics , 21, 2569-2583. https://doi.org/10.5194/acp-21-2569-2021
Khamala, G.W., Makokha, J.W., Boiyo, R. and Kumar, K.R. (2022) Long-Term Climatology and Spatial Trends of Absorption, Scattering, and Total Aerosol Optical Depths over East Africa during 2001-2019. Environmental Science and Pollution Research , 29, 61283-61297. https://doi.org/10.1007/s11356-022-20022-6
Aloysius, M., Mohan, M., Babu, S.S., Nair, V.S., Parameswaran, K. and Moorthy, K.K. (2008) Influence of Circulation Parameters on the AOD Variations over the Bay of Bengal during ICARB. Journal of Earth System Science , 117, 353-360. https://doi.org/10.1007/s12040-008-0038-6
Deng, X., Cao, W., Huo, Y., Yang, G., Yu, C., He, D., et al. (2018) Meteorological Conditions during a Severe, Prolonged Regional Heavy Air Pollution Episode in Eastern China from December 2016 to January 2017. Theoretical and Applied Climatology , 135, 1105-1122. https://doi.org/10.1007/s00704-018-2426-4
Guillén-Lambea, S., Carvalho, M., Delgado, M. and Lazaro, A. (2020) Sustainable Enhancement of District Heating and Cooling Configurations by Combining Thermal Energy Storage and Life Cycle Assessment. Clean Technologies and Environmental Policy , 23, 857-867. https://doi.org/10.1007/s10098-020-01941-9
Khamala, G.W. and Makokha, J.W. (2025) Spatiotemporal Variability and Source Apportionment of Particulate Matter (PM) Emissions Using Binned Size Distributions: Insights from MERRA-2 over Africa. Earth Systems and Environment . https://doi.org/10.1007/s41748-025-00641-y
Ramanathan, V., Crutzen, P.J., Kiehl, J.T. and Rosenfeld, D. (2001) Aerosols, Climate, and the Hydrological Cycle. Science , 294, 2119-2124. https://doi.org/10.1126/science.1064034
Satheesh, S. and Krishnamoorthy, K. (2005) Radiative Effects of Natural Aerosols: A Review. Atmospheric Environment , 39, 2089-2110. https://doi.org/10.1016/j.atmosenv.2004.12.029
Myhre, G. (2009) Consistency between Satellite-Derived and Modeled Estimates of the Direct Aerosol Effect. Science , 325, 187-190. https://doi.org/10.1126/science.1174461
Hansen, J., Sato, M. and Ruedy, R. (1997) Radiative Forcing and Climate Response. Journal of Geophysical Research : Atmospheres , 102, 6831-6864. https://doi.org/10.1029/96jd03436
Lee, K.H., Li, Z., Wong, M.S., Xin, J., Wang, Y., Hao, W., et al. (2007) Aerosol Single Scattering Albedo Estimated across China from a Combination of Ground and Satellite Measurements. Journal of Geophysical Research : Atmospheres , 112, D22S15. https://doi.org/10.1029/2007jd009077
Bahino, J., Giordano, M., Beekmann, M., Yoboué, V., Ochou, A., Galy-Lacaux, C., et al. (2024) Temporal Variability and Regional Influences of PM 2.5 in the West African Cities of Abidjan (Côte d’Ivoire) and Accra (Ghana). Environmental Science : Atmospheres , 4, 468-487. https://doi.org/10.1039/d4ea00012a
Sokolik, I.N. and Toon, O.B. (1999) Incorporation of Mineralogical Composition into Models of the Radiative Properties of Mineral Aerosol from UV to IR Wavelengths. Journal of Geophysical Research : Atmospheres , 104, 9423-9444. https://doi.org/10.1029/1998jd200048
Lyamani, H., Olmo, F.J. and Alados-Arboledas, L. (2009) Physical and Optical Properties of Aerosols over an Urban Location in Spain: Seasonal and Diurnal Variability. Atmospheric Chemistry and Physics , 9, 18159-18199. https://doi.org/10.5194/acpd-9-18159-2009
El-Metwally, M., Alfaro, S.C., Wahab, M.M.A., Favez, O., Mohamed, Z. and Chatenet, B. (2011) Aerosol Properties and Associated Radiative Effects over Cairo (Egypt). Atmospheric Research , 99, 263-276. https://doi.org/10.1016/j.atmosres.2010.10.017
Makokha, J.W. and Angeyo, H.K. (2013) Investigation of Radiative Characteristics of the Kenyan Atmosphere Due to Aerosols Using Sun Spectrophotometry Measurements and the COART Model. Aerosol and Air Quality Research , 13, 201-208. https://doi.org/10.4209/aaqr.2012.06.0146
Esteve, A.R., Estellés, V., Utrillas, M.P. and Martínez-Lozano, J.A. (2014) Analysis of the Aerosol Radiative Forcing over a Mediterranean Urban Coastal Site. Atmospheric Research , 137, 195-204. https://doi.org/10.1016/j.atmosres.2013.10.009
Kumar, S., Dey, S. and Srivastava, A. (2016) Quantifying Enhancement in Aerosol Radiative Forcing during “Extreme Aerosol Days” in Summer at Delhi National Capital Region, India. Science of the Total Environment , 550, 994-1000. https://doi.org/10.1016/j.scitotenv.2016.01.191
Kumar, K.R., Kang, N., Sivakumar, V. and Griffith, D. (2017) Temporal Characteristics of Columnar Aerosol Optical Properties and Radiative Forcing (2011-2015) Measured at AERONET’s Pretoria_CSIR_DPSS Site in South Africa. Atmospheric Environm ent , 165, 274-289. https://doi.org/10.1016/j.atmosenv.2017.06.048
Bibi, H., Alam, K., Blaschke, T., Bibi, S. and Iqbal, M.J. (2016) Long-Term (2007-2013) Analysis of Aerosol Optical Properties over Four Locations in the Indo-Gangetic Plains. Applied Optics , 55, 6199. https://doi.org/10.1364/ao.55.006199
Adesina, A.J., Kumar, K.R., Sivakumar, V. and Piketh, S.J. (2016) Intercomparison and Assessment of Long-Term (2004-2013) Multiple Satellite Aerosol Products over Two Contrasting Sites in South Africa. Journal of Atmospheric and Solar - Terrestrial Physics , 148, 82-95. https://doi.org/10.1016/j.jastp.2016.09.001
Khan, R., Kumar, K.R., Zhao, T. and Ali, G. (2020) The Contribution of Different Aerosol Types to Direct Radiative Forcing over Distinct Environments of Pakistan Inferred from the AERONET Data. Environmental Research Letters , 15, Article ID: 114062. https://doi.org/10.1088/1748-9326/aba2a6
Khamala, G.W., Makokha, J.W., Boiyo, R. and Kumar, K.R. (2023) Spatiotemporal Analysis of Absorbing Aerosols and Radiative Forcing over Environmentally Distinct Stations in East Africa during 2001-2018. Science of the Total Environment , 864, Article ID: 161041. https://doi.org/10.1016/j.scitotenv.2022.161041
Gauderman, W.J., Gilliland, G.F., Vora, H., Avol, E., Stram, D., McConnell, R., et al. (2002) Association between Air Pollution and Lung Function Growth in Southern California Children: Results from a Second Cohort. American Journal of Respiratory and Critical Care Medicine , 166, 76-84. https://doi.org/10.1164/rccm.2111021
Liao, W., Wang, X., Fan, Q., Zhou, S., Chang, M., Wang, Z., et al. (2015) Long-term Atmospheric Visibility, Sunshine Duration and Precipitation Trends in South China. Atmospheric Environment , 107, 204-216. https://doi.org/10.1016/j.atmosenv.2015.02.015
Yu, X., Kumar, K.R., Lü, R. and Ma, J. (2016) Changes in Column Aerosol Optical Properties during Extreme Haze-Fog Episodes in January 2013 over Urban Beijing. Environmental Pollution , 210, 217-226. https://doi.org/10.1016/j.envpol.2015.12.021
Mahowald, N., Albani, S., Kok, J.F., Engelstaeder, S., Scanza, R., Ward, D.S., et al. (2014) The Size Distribution of Desert Dust Aerosols and Its Impact on the Earth System. Aeolian Research , 15, 53-71. https://doi.org/10.1016/j.aeolia.2013.09.002
Jickells, T.D., An, Z.S., Andersen, K.K., Baker, A.R., Bergametti, G., Brooks, N., et al. (2005) Global Iron Connections between Desert Dust, Ocean Biogeochemistry, and Climate. Science , 308, 67-71. https://doi.org/10.1126/science.1105959
Wu, W., Purser, R.J. and Parrish, D.F. (2002) Three-Dimensional Variational Analysis with Spatially Inhomogeneous Covariances. Monthly Weather Review , 130, 2905-2916. https://doi.org/10.1175/1520-0493(2002)130<2905:tdvaws>2.0.co;2
Rienecker, M.M., Suarez, M.J., Gelaro, R., Todling, R., Bacmeister, J., Liu, E., et al. (2011) MERRA: Nasa’s Modern-Era Retrospective Analysis for Research and Applications. Journal of Climate , 24, 3624-3648. https://doi.org/10.1175/jcli-d-11-00015.1
Remer, L.A., Kaufman, Y.J., Tanré, D., Mattoo, S., Chu, D.A., Martins, J.V., et al. (2005) The MODIS Aerosol Algorithm, Products, and Validation. Journal of the Atmospheric Sciences , 62, 947-973. https://doi.org/10.1175/jas3385.1
Gelaro, R., McCarty, W., Suárez, M.J., Todling, R., Molod, A., Takacs, L., et al. (2017) The Modern-Era Retrospective Analysis for Research and Applications, Version 2 (MERRA-2). Journal of Climate , 30, 5419-5454. https://doi.org/10.1175/jcli-d-16-0758.1
Kok, J.F., Ward, D.S., Mahowald, N.M. and Evan, A.T. (2012) Global and Regional Importance of the Direct Dust-Climate Feedback. Nature Climate Change , 2, 437-445.
Ginoux, P., Prospero, J.M., Gill, T.E., Hsu, N.C. and Zhao, M. (2012) Global-Scale Attribution of Anthropogenic and Natural Dust Sources and Their Emission Rates Based on MODIS Deep Blue Aerosol Products. Reviews of Geophysics , 50, RG3005. https://doi.org/10.1029/2012rg000388
Eck, T.F., Holben, B.N., Reid, J.S., Arola, A., Ferrare, R.A., Hostetler, C.A., Sinyuk, A., et al. (2013) High Aerosol Absorption Optical Depths from Biomass Burning over the Southeast United States during the Summer of 2007: An Analysis Using Surface and Satellite Measurements. Journal of Geophysical Research : Atmospheres , 118, 12-205.
Evan, A.T., Flamant, C., Gaetani, M. and Guichard, F. (2016) The Past, Present and Future of African Dust. Science Advances , 2, e1500646.
Chatoutsidou, S.E., Diapouli, E., Manousakas, M., Vratolis, S., Maggos, T. and Eleftheriadis, K. (2019) Assessment of PM 10 -Bound Heavy Metals Seasonal Variation and Health Impact in Two Low Pollution Areas of Greece. Air Quality , Atmosphere & Health , 12, 547-558.
Gahungu, P., Kubwimana, J.R., Muhimpundu, L.J.M.B. AND Ndamuzi, E. (2022) Modelling Spatio-Temporal Trends of Air Pollution in Africa: A Case Study of PM 2.5 Variations across Different Regions. arXiv: 2208.12719.
Kalisa, E., Clark, M.L., Ntakirutimana, T., Amani, M. and Volckens, J. (2023) Exposure to Indoor and Outdoor Air Pollution in Schools in Africa: Current Status, Knowledge Gaps, and a Call to Action. Heliyon , 9, e18450. https://doi.org/10.1016/j.heliyon.2023.e18450
Mugagga, F., Nakanjakko, N., Nakileza, B. and Nseka, D. (2020) Vulnerability of Smallholder Sorghum Farmers to Climate Variability in a Heterogeneous Landscape of South-Western Uganda. Jàmbá Journal of Disaster Risk Studies , 12, a849. https://doi.org/10.4102/jamba.v12i1.849
Mutama, P.M., Makokha, J.W., Kelonye, F.B. and Khamala, G.W. (2024) Spatial-Temporal Assessment of Changes in Aerosol Optical Properties Pre, During, and Post COVID-19 Lockdowns over Kenya, East Africa. Open Access Library Journal , 11, e11223. https://doi.org/10.4236/oalib.1111223
Ngaina, J., Mutai, B., Ininda, J. and Muthama, J. (2014) Monitoring Spatial-Temporal Variability of Aerosol over Kenya. Ethiopian Journal of Environmental Studies and Management , 7, 244-252. https://doi.org/10.4314/ejesm.v7i3.3
Ongoma, V. and Chen, H. (2016) Temporal and Spatial Variability of Temperature and Precipitation over East Africa from 1951 to 2010. Meteorology and Atmospheric Physics , 129, 131-144. https://doi.org/10.1007/s00703-016-0462-0
Makokha, J.W., Odhiambo, J.O. and Shem, J.G. (2018) Long Term Assessment of Aerosol Radiative Forcing over Selected Sites of East Africa. Journal of Geoscience and Environment Protection , 6, 22-34. https://doi.org/10.4236/gep.2018.64002
Boiyo, R., Kumar, K.R. and Zhao, T. (2018) Spatial Variations and Trends in AOD Climatology over East Africa during 2002-2016: A Comparative Study Using Three Satellite Data Sets. International Journal of Climatology , 38, e1221-e1240. https://doi.org/10.1002/joc.5446
Kaufman, Y.J., Koren, I., Remer, L.A., Rosenfeld, D. and Rudich, Y. (2005) The Effect of Smoke, Dust, and Pollution Aerosol on Shallow Cloud Development over the Atlantic Ocean. Proceedings of the National Academy of Sciences of the United States of America , 102, 11207-11212. https://doi.org/10.1073/pnas.0505191102
Hsu, N.C., Jeong, M.‐., Bettenhausen, C., Sayer, A.M., Hansell, R., Seftor, C.S., et al. (2013) Enhanced Deep Blue Aerosol Retrieval Algorithm: The Second Generation. Journal of Geophysical Research : Atmospheres , 118, 9296-9315. https://doi.org/10.1002/jgrd.50712
Sayer, A.M., Hsu, N.C., Bettenhausen, C. and Jeong, M. (2013) Validation and Uncertainty Estimates for MODIS Collection 6 “Deep Blue” Aerosol Data. Journal of Geophysical Research : Atmospheres , 118, 7864-7872. https://doi.org/10.1002/jgrd.50600
Sayer, A.M., Munchak, L.A., Hsu, N.C., Levy, R.C., Bettenhausen, C. and Jeong, M. (2014) MODIS Collection 6 Aerosol Products: Comparison between Aqua’s E-Deep Blue, Dark Target, and “Merged” Data Sets, and Usage Recommendations. Journal of Geophysical Research : Atmospheres , 119, 13965-13989. https://doi.org/10.1002/2014jd022453
Levy, R.C., Remer, L.A., Kleidman, R.G., Mattoo, S., Ichoku, C., Kahn, R., et al. (2010) Global Evaluation of the Collection 5 MODIS Dark-Target Aerosol Products over Land. Atmospheric Chemistry and Physics , 10, 10399-10420. https://doi.org/10.5194/acp-10-10399-2010
Smirnov, A., Holben, B.N., Eck, T.F., Slutsker, I., Chatenet, B. and Pinker, R.T. (2000) Aerosol Optical Depth Measurements during the Aerosols99 Experiment. Journal of Geophysical Research : Atmospheres , 105, 15127-15138.
Eck, T.F., Holben, B.N., Sinyuk, A., Pinker, R.T., Goloub, P., Chen, H., et al. (2010) Climatological Aspects of the Optical Properties of Fine/Coarse Mode Aerosol Mixtures. Journal of Geophysical Research : Atmospheres , 115, D19205. https://doi.org/10.1029/2010jd014002
Khamala, G.W., Odhiambo, J.O. and Makokha, J.W. (2018) Seasonal Variability in Aerosol Microphysical Properties over Selected Rural, Urban and Maritime Sites in Kenya. Open Access Library Journal , 5, e4821. https://doi.org/10.4236/oalib.1104821
Miller, R.L., Tegen, I. and Perlwitz, J. (2004) Surface Radiative Forcing by Soil Dust Aerosols and the Hydrologic Cycle. Journal of Geophysical Research : Atmospheres , 109, D04203. https://doi.org/10.1029/2003jd004085
Makokha, J., Masayi, N., Barasa, P., Ikoha, P., Konje, M., Mutonyi, J., et al. (2024) Assessing the Long-Term Changes in Selected Meteorological Parameters over the North-Rift, Kenya: A Regional Climatology Perspective. Hydrology , 12, 59-76. https://doi.org/10.11648/j.hyd.20241203.12
Khamala, G.W., Makokha, J.W. and Boiyo, R. (2024) The Spatiotemporal and Dependency Analysis of Selected Meteorological Parameters and Normalized Difference Vegetation Index with Aerosol Optical Depth over East Africa. Heliyon , 10, e39961. https://doi.org/10.1016/j.heliyon.2024.e39961