Coordination Interaction between Rare Earth and/or Transition Metal Centers and Thiophene Series Oligomer Derivatives in Ultrathin Langmuir-Blodgett Films — Oak Academic Publishing
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Coordination Interaction between Rare Earth and/or Transition Metal Centers and Thiophene Series Oligomer Derivatives in Ultrathin Langmuir-Blodgett Films
Physics Department, Belarusian State University, Minsk, Belarus
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Physics Department, Belarusian State University, Minsk, Belarus
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Belarusian State University of Informatics and Radioelectronics, Minsk, Belarus
1 Physics Department, Belarusian State University, Minsk, Belarus
2 Physics Department, Belarusian State University, Minsk, Belarus
3 Belarusian State University of Informatics and Radioelectronics, Minsk, Belarus
It has been shown by thermodynamic and electro-chemical methods that coordination interactions are involved in the process of incorporation of rare-earth elements and/or Fe into Langmuir monolayers of oligomer with alkyl fragment. A coordination mechanism, which is responsible for self-organization of octahedral Fe(II) - complexes of nano-cyclic ligands obtained from oligomer of thiophene pyrrole series derivatives in compressed Langmuir monolayers has been proposed. It has been established that a coordinational-polymeric hexagonal network of nano-cyclic ligands with metal centers is formed at the phase transition when compressing the Langmuir monolayers of thiophene pyrrole series oligomer with alkyl fragment on surface of subphase with rare-earth (Sm, Er, Ce) and/or Fe ions.
KeywordsLangmuir MonolayerSelf-OrganizationMetal-Containing Ultrathin Langmuir-Blodgett Film
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